10,281 research outputs found
Soft Manifold Dynamics Behind Negative Thermal Expansion
Minimal models are developed to examine the origin of large negative thermal
expansion (NTE) in under-constrained systems. The dynamics of these models
reveals how underconstraint can organize a thermodynamically extensive manifold
of low-energy modes which not only drives NTE but extends across the Brillioun
zone. Mixing of twist and translation in the eigenvectors of these modes, for
which in ZrW2O8 there is evidence from infrared and neutron scattering
measurements, emerges naturally in our model as a signature of the dynamics of
underconstraint.Comment: 5 pages, 3 figure
Ordered Phase of the Dipolar Spin Ice under [110]-Magnetic Fields
We find that the true ground state of the dipolar spin ice system under
[110]-magnetic fields is the ``Q=X'' structure, which is consistent with both
experiments and Monte Carlo simulations. We then perform a Monte Carlo
simulation to confirm that there exists a first order phase transition under
the [110]-field. In particular this result indicates the existence of the first
order phase transition to the ``Q=X'' phase in the field above 0.35 T for
Dy2Ti2O7. We also show the magnetic field-temperature phase diagram to
summarize the ordered states of this system.Comment: 4 pages, 5 figures, in RevTex4, submitted to J. Phys. Soc. Jp
Separating extended disc features from the protoplanet in PDS 70 using VLT/SINFONI
Transition discs are prime targets to look for protoplanets and study
planet-disc interactions. We present VLT/SINFONI observations of PDS~70, a
transition disc with a recently claimed embedded protoplanet. We take advantage
of the angular and spectral diversity present in our data for an optimal PSF
modeling and subtraction using principal component analysis (PCA). We report
the redetection of PDS 70 b, both the front and far side of the outer disc
edge, and the detection of several extended features in the annular gap. We
compare spectral differential imaging applied before (PCA-SADI), and after
(PCA-ASDI) angular differential imaging. Our tests suggest that PCA-SADI better
recovers extended features, while PCA-ASDI is more sensitive to point sources.
We adapted the negative fake companion (NEGFC) technique to infer the
astrometry of the companion, and derived and
PA = 158.7deg 3.0deg. We used both NEGFC and ANDROMEDA to infer the
-band spectro-photometry of the protoplanet, and found results consistent
with recent VLT/SPHERE observations, except for their 2018/02 epoch measurement
in the filter. Finally, we derived an upper limit of yr for the accretion rate of the companion
based on an adaptation of PCA-SADI/PCA-ASDI around the Br line.Comment: 20 pages, 12 figures. This is a pre-copyedited, author-produced PDF
of an article accepted for publication in MNRAS on 2019 April 2
Pyramidal micromirrors for microsystems and atom chips
Concave pyramids are created in the (100) surface of a silicon wafer by anisotropic etching in potassium hydroxide. High quality micromirrors are then formed by sputtering gold onto the smooth silicon (111) faces of the pyramids. These mirrors show great promise as high quality optical devices suitable for integration into micro-optoelectromechanical systems and atom chips. We have shown that structures of this shape can be used to laser-cool and hold atoms in a magneto-optical trap
Spin ice in a field: quasi-phases and pseudo-transitions
Thermodynamics of the short-range model of spin ice magnets in a field is
considered in the Bethe - Peierls approximation. The results obtained for
[111], [100] and [011] fields agrees reasonably well with the existing
Monte-Carlo simulations and some experiments. In this approximation all
extremely sharp field-induced anomalies are described by the analytical
functions of temperature and applied field. In spite of the absence of true
phase transitions the analysis of the entropy and specific heat reliefs over
H-T plane allows to discern the "pseudo-phases" with specific character of spin
fluctuations and define the lines of more or less sharp "pseudo-transitions"
between them.Comment: 18 pages, 16 figure
Dynamic Approach to the Fully Frustrated XY Model
Using Monte Carlo simulations, we systematically investigate the
non-equilibrium dynamics of the chiral degree of freedom in the two-dimensional
fully frustrated XY model. The critical initial increase of the staggered
chiral magnetization is observed. By means of the short-time dynamics approach,
we estimate the second order phase transition temperature and all the
dynamic and static critical exponents , z, and .Comment: 5 pages with 6 figures include
Voltage-controlled current loops with nanofluidic diodes electrically coupled to solid state capacitors
[EN] We describe experimentally and theoretically voltage-controlled current loops obtained with nanofluidic diodes immersed in aqueous salt solutions. The coupling of these soft matter diodes with conventional electronic elements such as capacitors permits simple equivalent circuits which show electrical properties reminiscent of a resistor with memory. Different conductance levels can be reproducibly achieved under a wide range of experimental conditions (input voltage amplitudes and frequencies, load capacitances, electrolyte concentrations, and single pore and multipore membranes) by electrically coupling two types of passive components: the nanopores (ionics) and the capacitors (electronics). Remarkably, these electrical characteristics do not result from slow ionic redistributions within the nanopores, which should be difficult to control and would give only small conductance changes, but arise from the robust collective response of equivalent circuits. Coupling nanoscale diodes with conventional electronic elements allows interconverting ionic and electronic currents, which should be useful for electrochemical signal processing and energy conversion based on charge transport.Support from the Ministry of Economic Affairs and Competitiveness and FEDER (project MAT2015-65011-P), the Generalitat Valenciana (project Prometeo/GV/0069 for Groups of Excellence). M. A, S. N. and W. E acknowledge the funding from the Hessen State Ministry of Higher Education, Research and the Arts, Germany, in the frame of LOEWE project iNAPO. Z. S. acknowledges the funding from the National Science Foundation (CHE 1306058).Ramirez Hoyos, P.; Gómez Lozano, V.; Cervera, J.; Nasir, S.; Ali, M.; Ensinger, W.; Siwy, Z.... (2016). Voltage-controlled current loops with nanofluidic diodes electrically coupled to solid state
capacitors. RSC Advances. 6(60):54742-54746. https://doi.org/10.1039/c6ra08277gS5474254746660Fologea, D., Krueger, E., Mazur, Y. I., Stith, C., Okuyama, Y., Henry, R., & Salamo, G. J. (2011). Bi-stability, hysteresis, and memory of voltage-gated lysenin channels. Biochimica et Biophysica Acta (BBA) - Biomembranes, 1808(12), 2933-2939. doi:10.1016/j.bbamem.2011.09.005Pustovoit, M. A., Berezhkovskii, A. M., & Bezrukov, S. M. (2006). Analytical theory of hysteresis in ion channels: Two-state model. The Journal of Chemical Physics, 125(19), 194907. doi:10.1063/1.2364898Ramirez, P., Cervera, J., Ali, M., Ensinger, W., & Mafe, S. (2014). Logic Functions with Stimuli-Responsive Single Nanopores. ChemElectroChem, 1(4), 698-705. doi:10.1002/celc.201300255Martin, C. R., & Siwy, Z. S. (2007). CHEMISTRY: Learning Nature’s Way: Biosensing with Synthetic Nanopores. Science, 317(5836), 331-332. doi:10.1126/science.1146126Hou, X., & Jiang, L. (2009). Learning from Nature: Building Bio-Inspired Smart Nanochannels. ACS Nano, 3(11), 3339-3342. doi:10.1021/nn901402bZhang, H., Tian, Y., & Jiang, L. (2016). Fundamental studies and practical applications of bio-inspired smart solid-state nanopores and nanochannels. Nano Today, 11(1), 61-81. doi:10.1016/j.nantod.2015.11.001Chun, H., & Chung, T. D. (2015). Iontronics. Annual Review of Analytical Chemistry, 8(1), 441-462. doi:10.1146/annurev-anchem-071114-040202Tagliazucchi, M., & Szleifer, I. (2015). Transport mechanisms in nanopores and nanochannels: can we mimic nature? Materials Today, 18(3), 131-142. doi:10.1016/j.mattod.2014.10.020Misra, N., Martinez, J. A., Huang, S.-C. J., Wang, Y., Stroeve, P., Grigoropoulos, C. P., & Noy, A. (2009). Bioelectronic silicon nanowire devices using functional membrane proteins. Proceedings of the National Academy of Sciences, 106(33), 13780-13784. doi:10.1073/pnas.0904850106Senapati, S., Basuray, S., Slouka, Z., Cheng, L.-J., & Chang, H.-C. (2011). A Nanomembrane-Based Nucleic Acid Sensing Platform for Portable Diagnostics. Topics in Current Chemistry, 153-169. doi:10.1007/128_2011_142Haywood, D. G., Saha-Shah, A., Baker, L. A., & Jacobson, S. C. (2014). Fundamental Studies of Nanofluidics: Nanopores, Nanochannels, and Nanopipets. Analytical Chemistry, 87(1), 172-187. doi:10.1021/ac504180hPérez-Mitta, G., Tuninetti, J. S., Knoll, W., Trautmann, C., Toimil-Molares, M. E., & Azzaroni, O. (2015). Polydopamine Meets Solid-State Nanopores: A Bioinspired Integrative Surface Chemistry Approach To Tailor the Functional Properties of Nanofluidic Diodes. Journal of the American Chemical Society, 137(18), 6011-6017. doi:10.1021/jacs.5b01638Ali, M., Nasir, S., Ramirez, P., Ahmed, I., Nguyen, Q. H., Fruk, L., … Ensinger, W. (2011). Optical Gating of Photosensitive Synthetic Ion Channels. Advanced Functional Materials, 22(2), 390-396. doi:10.1002/adfm.201102146Ali, M., Nasir, S., Ramirez, P., Cervera, J., Mafe, S., & Ensinger, W. (2013). Carbohydrate-Mediated Biomolecular Recognition and Gating of Synthetic Ion Channels. The Journal of Physical Chemistry C, 117(35), 18234-18242. doi:10.1021/jp4054555Ali, M., Ahmed, I., Nasir, S., Ramirez, P., Niemeyer, C. M., Mafe, S., & Ensinger, W. (2015). Ionic Transport through Chemically Functionalized Hydrogen Peroxide-Sensitive Asymmetric Nanopores. ACS Applied Materials & Interfaces, 7(35), 19541-19545. doi:10.1021/acsami.5b06015Albrecht, T. (2011). How to Understand and Interpret Current Flow in Nanopore/Electrode Devices. ACS Nano, 5(8), 6714-6725. doi:10.1021/nn202253zLemay, S. G. (2009). Nanopore-Based Biosensors: The Interface between Ionics and Electronics. ACS Nano, 3(4), 775-779. doi:10.1021/nn900336jGomez, V., Ramirez, P., Cervera, J., Nasir, S., Ali, M., Ensinger, W., & Mafe, S. (2015). Charging a Capacitor from an External Fluctuating Potential using a Single Conical Nanopore. Scientific Reports, 5(1). doi:10.1038/srep09501Ramirez, P., Gomez, V., Cervera, J., Nasir, S., Ali, M., Ensinger, W., & Mafe, S. (2015). Energy conversion from external fluctuating signals based on asymmetric nanopores. Nano Energy, 16, 375-382. doi:10.1016/j.nanoen.2015.07.013Tybrandt, K., Forchheimer, R., & Berggren, M. (2012). Logic gates based on ion transistors. Nature Communications, 3(1). doi:10.1038/ncomms1869Apel, P. (2001). Track etching technique in membrane technology. Radiation Measurements, 34(1-6), 559-566. doi:10.1016/s1350-4487(01)00228-1Cervera, J., Schiedt, B., Neumann, R., Mafé, S., & Ramírez, P. (2006). Ionic conduction, rectification, and selectivity in single conical nanopores. The Journal of Chemical Physics, 124(10), 104706. doi:10.1063/1.2179797Ali, M., Ramirez, P., Mafé, S., Neumann, R., & Ensinger, W. (2009). A pH-Tunable Nanofluidic Diode with a Broad Range of Rectifying Properties. ACS Nano, 3(3), 603-608. doi:10.1021/nn900039fRamirez, P., Gomez, V., Verdia-Baguena, C., Nasir, S., Ali, M., Ensinger, W., & Mafe, S. (2016). Designing voltage multipliers with nanofluidic diodes immersed in aqueous salt solutions. Physical Chemistry Chemical Physics, 18(5), 3995-3999. doi:10.1039/c5cp07203dWang, D., Kvetny, M., Liu, J., Brown, W., Li, Y., & Wang, G. (2012). Transmembrane Potential across Single Conical Nanopores and Resulting Memristive and Memcapacitive Ion Transport. Journal of the American Chemical Society, 134(8), 3651-3654. doi:10.1021/ja211142eMomotenko, D., & Girault, H. H. (2011). Scan-Rate-Dependent Ion Current Rectification and Rectification Inversion in Charged Conical Nanopores. Journal of the American Chemical Society, 133(37), 14496-14499. doi:10.1021/ja2048368Zhang, A., & Lieber, C. M. (2015). Nano-Bioelectronics. Chemical Reviews, 116(1), 215-257. doi:10.1021/acs.chemrev.5b0060
Competing Magnetic Phases on a "Kagome Staircase"
We present thermodynamic and neutron data on Ni_3V_2O_8, a spin-1 system on a
kagome staircase. The extreme degeneracy of the kagome antiferromagnet is
lifted to produce two incommensurate phases at finite T - one amplitude
modulated, the other helical - plus a commensurate canted antiferromagnet for T
->0. The H-T phase diagram is described by a model of competing first and
second neighbor interactions with smaller anisotropic terms. Ni_3V_2O_8 thus
provides an elegant example of order from sub leading interactions in a highly
frustrated systemComment: 4 pages, 3 figure
Universal Short-time Behaviour of the Dynamic Fully Frustrated XY Model
With Monte Carlo methods we investigate the dynamic relaxation of the fully
frustrated XY model in two dimensions below or at the Kosterlitz-Thouless phase
transition temperature. Special attention is drawn to the sublattice structure
of the dynamic evolution. Short-time scaling behaviour is found and
universality is confirmed. The critical exponent is measured for
different temperature and with different algorithms.Comment: 18 pages, LaTeX, 8 ps-figure
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